An excellent live Will-Sheff-only version of Okkervil River's "A Girl in Port"...
Introduce yourself to the Black Swans (MySpace). I like what I've heard. Same goes for the jazz of Anat Cohen (MySpace).
Black Moth Super Rainbow's Dandelion Gum (MySpace) is really, really good psychedelic folksy pop. Pitchfork thinks so too. "Sun Lips"...
Caribou's Andorra is my introduction to this excellent band (MySpace). The album is captivating. "Melody Day"...
Check out this mini documentary on the making of Andorra...
Also be sure to check out their live video collection of all songs from Andorra.